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Research Progress of Cellulose-based Gel Polymer Electrolytes for Lithium Batteries
Received:June 09, 2023  
DOI:10.11981/j.issn.1000-6842.2023.03.01
Key Words:cellulose;lithium batteries;gel polymer electrolyte;lithium dendrite
Fund Project:国家自然科学基金(22378247);生物质化学与材料国际联合研究中心(2018GHJD-19);陕西省重点产业创新链项目(2020ZDLGY11-03);中国-中东欧国家高校联合教育项目(2021099)。
Author NameAffiliationE-mail
ZHANG Sufeng* College of Bioresources Chemical and Materials Engineering, Shaanxi University of Science & Technology, Xi’an, Shaanxi Province, 710021 zhangsufeng@sust.edu.cn 
DENG Tingting College of Bioresources Chemical and Materials Engineering, Shaanxi University of Science & Technology, Xi’an, Shaanxi Province, 710021  
LI Lei College of Bioresources Chemical and Materials Engineering, Shaanxi University of Science & Technology, Xi’an, Shaanxi Province, 710021  
ZHU Xinyue College of Bioresources Chemical and Materials Engineering, Shaanxi University of Science & Technology, Xi’an, Shaanxi Province, 710021  
LIU Yali College of Bioresources Chemical and Materials Engineering, Shaanxi University of Science & Technology, Xi’an, Shaanxi Province, 710021  
LI Nan College of Bioresources Chemical and Materials Engineering, Shaanxi University of Science & Technology, Xi’an, Shaanxi Province, 710021  
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Abstract:
      Electrolyte, as one of the main components of lithium batteries, plays an important role in the transport of lithium ions during the charging and discharging process. However, the frequent safety accidents caused by problems such as traditional liquid electrolyte leakage and lithium dendrite growth during charging and discharging seriously limit the wide applications of lithium batteries. Compared with liquid electrolytes, gel polymer electrolytes (GPE) integrate the separate with the liquid electrolyte, and overall improved safety performance and electrochemical performance. Because of its excellent thermal stability, good mechanical properties and strong electrolyte affinity, cellulose has received extensive attention in the field of GPE research in recent years. In this paper, the current research progress of micro-cellulose, nano-cellulose, regenerated cellulose and cellulose derivatives in the field of GPE is reviewed, and the effects of different cellulose matrices or functional fillers on the properties of GPE composite are analyzed, and finally the challenges of cellulose-based GPE in high-performance lithium batteries are proposed, and their research prospects are prospected.
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