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Research Progress of Cellulose-based Solid-state Electrolytes in All-solid-state Lithium Metal Batteries
Received:May 29, 2026  Revised:June 25, 2026
DOI：10.11981/j.issn.1000-6842.2026.03.188
Key Words:cellulose;solid-state electrolyte;all-solid-state battery;ion transport
Fund Project:国家自然科学基金22308176山东省重大科技创新工程（山东省重点研发计划）2024CXGC010702中央引导地方科技发展资金YDZX2025114山东省高等学校青年创新团队发展计划2024KJN016国家自然科学基金（22308176）；山东省重大科技创新工程（山东省重点研发计划）（2024CXGC010702）；中央引导地方科技发展资金（YDZX2025114）；山东省高等学校青年创新团队发展计划（2024KJN016）。
Author NameAffiliationPostcode
Cao Jiangqing* 1Key Lab of Advanced Glass Manufacturing and Processing Technology of Shandong Province， Collaborative Innovation Center for Green and Low-carbon Materials for Ecological Protection and High-quality Development in the Yellow River Basin， Qilu University of Technology （Shandong Academy of Sciences）， Ji’nan， Shandong Province， 250353 250353
Zhao Wenquan 1Key Lab of Advanced Glass Manufacturing and Processing Technology of Shandong Province， Collaborative Innovation Center for Green and Low-carbon Materials for Ecological Protection and High-quality Development in the Yellow River Basin， Qilu University of Technology （Shandong Academy of Sciences）， Ji’nan， Shandong Province， 250353 250353
Zhang Jing 1Key Lab of Advanced Glass Manufacturing and Processing Technology of Shandong Province， Collaborative Innovation Center for Green and Low-carbon Materials for Ecological Protection and High-quality Development in the Yellow River Basin， Qilu University of Technology （Shandong Academy of Sciences）， Ji’nan， Shandong Province， 250353 250353
Sun Peipei 1Key Lab of Advanced Glass Manufacturing and Processing Technology of Shandong Province， Collaborative Innovation Center for Green and Low-carbon Materials for Ecological Protection and High-quality Development in the Yellow River Basin， Qilu University of Technology （Shandong Academy of Sciences）， Ji’nan， Shandong Province， 250353 250353
Li Yong 1Key Lab of Advanced Glass Manufacturing and Processing Technology of Shandong Province， Collaborative Innovation Center for Green and Low-carbon Materials for Ecological Protection and High-quality Development in the Yellow River Basin， Qilu University of Technology （Shandong Academy of Sciences）， Ji’nan， Shandong Province， 250353 250353
Li Dongwei 1Key Lab of Advanced Glass Manufacturing and Processing Technology of Shandong Province， Collaborative Innovation Center for Green and Low-carbon Materials for Ecological Protection and High-quality Development in the Yellow River Basin， Qilu University of Technology （Shandong Academy of Sciences）， Ji’nan， Shandong Province， 250353 250353
Jia Mengying* 2School of Municipal and Environmental Engineering， Shandong Jianzhu University， Ji’nan， Shandong Province， 250101 250101
Wang Meng* 1Key Lab of Advanced Glass Manufacturing and Processing Technology of Shandong Province， Collaborative Innovation Center for Green and Low-carbon Materials for Ecological Protection and High-quality Development in the Yellow River Basin， Qilu University of Technology （Shandong Academy of Sciences）， Ji’nan， Shandong Province， 250353 250353
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Abstract:
      The development of cellulose-based solid-state electrolytes that combine environmental friendliness， high ionic conductivity， excellent interfacial stability， and high mechanical strength， is a key research direction in the field of all-solid-state lithium metal batteries. This paper focused on recent research progress regarding cellulose-based solid-state electrolytes in all-solid-state lithium metal batteries， providing a detailed review of their mechanisms of action in ion transport， interfacial stability， and mechanical reinforcement. It systematically outlined the mainstream preparation processes for cellulose-based solid-state electrolytes， including solution casting， hot-pressing， electrospinning， and in-situ polymerization， and summarized the structural design concepts and performance optimization strategies for cellulose-based solid-state electrolytes， such as cellulose and its derivatives， cellulose/polymer composite systems， and cellulose/inorganic composite systems， etc. Additionally， this paper systematically analyzed the current technical bottlenecks facing the application of cellulose-based solid-state electrolytes and provided an outlook on their future development trends and research directions.
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